`First Declaration of Mr. William C. Jones
`
`UNITED STATES PATENT AND TRADEMARK OFFICE
`_______________
`
`BEFORE THE PATENT TRIAL AND APPEAL BOARD
`_____________
`
`DAICEL CORPORATION
`Petitioner
`v.
`
`CELANESE INTERNATIONAL CORPORATION
`Patent Owner
`
`Patent No. 8,076,507
`Issue Date: Dec 13, 2011
`Title: REMOVAL OF PERMANGANATE REDUCING COMPOUNDS FROM
`METHANOL CARBONYLATION PROCESS STREAM
`
`Inter Partes Review No. 2015-00171
`____________________________________________________________
`
`FIRST DECLARATION OF WILLIAM C. JONES
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`(cid:44)(cid:51)(cid:53)(cid:3)(cid:49)(cid:82)(cid:17)(cid:3)(cid:21)(cid:19)(cid:20)(cid:24)(cid:16)(cid:19)(cid:19)(cid:20)(cid:26)(cid:20)
`(cid:40)(cid:91)(cid:75)(cid:76)(cid:69)(cid:76)(cid:87)(cid:3)(cid:20)(cid:19)(cid:22)(cid:28)
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`Patent No. 8,076,507
`First Declaration of Mr. William C. Jones
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`I, William C. Jones, hereby declare and say that:
`
`I. Introduction
`
`1.
`
`I am a chemical engineer, currently retired from Eastman Chemical
`
`Company.
`
`2.
`
`I have more than 40 years of experience in industrial-scale chemical
`
`processing, including the industrial-scale production of acetic acid and acetic
`
`anhydride. A copy of my curriculum vitae is attached as Exhibit 1038.
`
`3.
`
`I am very familiar with the subject matter of industrial-scale distillations and
`
`separations, in general. Most of my career at Eastman Chemical was involved
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`in R&D and operations management for production of acetic acid and acetyl
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`derivatives. This included pilot plant operation for production of acetic acid
`
`via methyl acetate carbonylation, and the design, construction,
`
`commissioning, and operation of acetic acid plants for Eastman and later for
`
`SIPCHEM (Saudi International Petrochemical Company). I also led process
`
`improvement and development efforts for the acetyl processes at Eastman and
`
`SIPCHEM. I was the Technology Director for the development of a nickel
`
`catalyzed methanol carbonylation technology. The last 5 years of my career
`
`at Eastman were spent in Eastman’s licensing group as Director of
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`Patent No. 8,076,507
`First Declaration of Mr. William C. Jones
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`Technology. During this time, the licensing of acetic acid technology was a
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`major focus of my work. My evaluation of projects included the technical
`
`aspects, as well as economic, financial and business evaluations comparing
`
`Eastman technology with other acetic acid technologies.
`
`4.
`
`I am named inventor on two patents/patent applications, both involving the
`
`process of methanol carbonylation. A listing of my patents and patent
`
`applications is included with my CV. These are relevant because they relate
`
`to and partially describe my experience and expertise in the field of the
`
`production and purification of acetic acid and acetic anhydride.
`
`5.
`
`I have been retained by the law firm of Foley & Lardner LLP, counsel for
`
`Daicel Corporation, to consult with legal counsel, to prepare this and
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`potentially other declarations, and to be available to testify in this matter. In
`
`providing expert consulting services in this matter, I am being paid at a rate of
`
`$175/hour for time spent on this matter, and I am being reimbursed for actual
`
`expenses. My compensation in no way depends upon the outcome of this
`
`inter partes reexamination proceeding, or any other proceeding before the US
`
`Patent and Trademark Office, or matter in litigation.
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`6.
`
`I have considered the following documents in forming my opinions:
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`000003
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`Patent No. 8,076,507
`First Declaration of Mr. William C. Jones
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`1013
`
`1014
`
`1015
`1016
`1017
`
`Exhibit No. Document
`1002
`U.S. Patent No. 8,076,507 (“the ’507 Patent”)
`First Declaration of Jeremy Cooper
`1003
`Curriculum Vitae for Jeremy Cooper
`1004
`1005
`Declaration of Mr. Hiroyuki Miura (“the Miura Decl.”)
`1006
`Résumé of Mr. Hiroyuki Miura.
`1007
`U.S. Patent Appl. 10/708,420 (“the ’420 Application”)
`1008
`U.S. Patent Appl. 11/788,455 (“the ’455 Application”)
`1009
`Applicant’s Response of January 6, 2011 in the ’455 Application
`1010
`U.S. Patent No. 5,625,095 (“the ’095 Patent”)
`1011
`U.S. Patent No. 6,339,171 (“the ’171 Patent”)
`Akinori, S. “Acetic Acid Synthesis From Methanol” J. Japan
`1012
`Petroleum Institute 20(5); 379-462 (1977)
`Certified English Translation of Akinori, S. “Acetic Acid
`Synthesis From Methanol” J. Japan Petroleum Institute 20(5);
`379-462 (1977) (“Akinori Translation”)
`European Patent Application Publication No. 1720821 (“EP
`’821”)
`Annex 3 as submitted in EP’821 (“Annex 3”)
`European Patent No. 0687662 A2
`Perry’s Chemical Engineers’ Handbook, Sixth Edition, 1984,
`pages 3-25 to 3-63.
`Oxford English Dictionary, second edition, 2002.
`Japanese Patent Application No. 2000-72712 (“JP 2000-72712”)
`Certified English Translation of JP 2000-72712 (“JP ’712”)
`Copy of http://www.rb-e.com/s/iodine-industry.asp as obtained
`on September 3, 2014.
`Interlocutory decision rendered by the Opposition Board in
`European Patent Application No. 05723599.6
`European Patent Application No. 05723599.6
`U.S. Patent No. 7,223,833
`Experiment results “D6” submitted by Daicel in opposition
`proceedings in European Patent Application No. 05723599.6
`Experiment results “D7” submitted by Daicel in opposition
`proceedings in European Patent Application No. 05723599.6
`Celanese Response as filed in the ’455 Application on July 7,
`2011
`Morello et al. “Commercial Extraction Equipment” Absorption
`
`1018
`1019
`1020
`1021
`
`1022
`
`1023
`1024
`1025
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`1026
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`1027
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`1028
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`Patent No. 8,076,507
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`and Extraction Sixteenth Annual Chemical Engineering
`Symposium 42(6); 1021-1035 (1950).
`
`1029
`1030
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`Sander, S. et al. Chem. Eng. Res. and Design. 85(1): 149-154.
`Diep, B.T. et al. J. Chem. Eng. Data. 32(3); 330-333 (1987).
`
`
`
`I have also reviewed the following documents, which I understand were
`
`previously prepared and served on the opposing party in this proceeding: (i)
`
`the Supplemental Declaration of Jeremy Cooper; (ii) an excerpt from the
`
`Minerals Yearbook 2000; (iii) an excerpt from Fundamentals of Chemistry,
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`Third Edition; (iv) a printout of the webpage at
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`http://www.chemguide.co.uk/physical/equilibria/kc.html; and (v) an excerpt
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`from Perry’s Chemical Engineers’ Handbook, Sixth Edition.
`
`Testimony Relevant To The Claims Of The ’507 Patent
`
`7.
`
`I am informed that Celanese International Corporation filed U.S. Patent
`
`Application No. 10/708,420 (Ex 1007; “the ’420 Application”) on March 2,
`
`2004, on April 20, 2007 U.S. Patent Application No. 11/788,455 (Ex 1008;
`
`“the ’455 Application”) was filed as a continuing application, and that on
`
`December 13, 2011 U.S. Patent No. 8,076,507 (Ex 1002; “the ‘507 Patent”)
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`issued therefrom. I understand that the named inventors of the ’507 Patent are
`
`Mark O. Scates, David A. Trueba, and Raymond J. Zinobile. I will refer
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`herein to the applicant of, and the named inventors in, the ’507 Patent
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`collectively as “Celanese.”
`
`8.
`
`I am informed that only claims 42-44, 47-51, 53 and 55-57 of the ’507 Patent
`
`are involved in this proceeding. Where appropriate, I will refer to these
`
`claims as either “the claims,” or the “Celanese claims.”
`
`9.
`
`Generally speaking, claims 42-44, 47-51, 53 and 55-57 are directed to a
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`process for separating a mixture comprising water, acetic acid, methyl iodide,
`
`methyl acetate, methanol, and at least one permanganate reducing compound
`
`(PRC), where the process includes the steps of (a) distilling the mixture to
`
`separate the mixture into a plurality of streams, at least one of said streams
`
`being a PRC enriched overhead stream comprising dimethyl ether (“DME”);
`
`and (b) extracting the PRC enriched overhead stream with water to produce an
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`aqueous stream comprising said at least one PRC, and a raffinate stream
`
`comprising methyl iodide. The distilling step separates the mixture
`
`comprising water, acetic acid, methyl iodide, methyl acetate, methanol, and at
`
`least one PRC into a “PRC enriched overhead stream” that contains DME and
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`a PRC. See the ’507 Patent, claim 42. This PRC enriched overhead stream is
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`then extracted with water to create an aqueous stream comprising at least one
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`PRC and a raffinate. Id. The extracting step also must include at least one of
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`three “wherein” clauses in claim 42. The first two “wherein” clauses each
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`require that at least two consecutive extraction steps be performed; the
`
`difference being the first requires a fresh water stream to be used in each
`
`discrete extraction stage and the second requires a single water stream to pass
`
`through each of the discrete extraction stages in series. Id. The third
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`“wherein” clause requires use of a continuous contacting extractor rather than
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`two consecutive extraction steps. Id.
`
`10.
`
`I have reviewed claims 42-44, 47-51, 53, 55, and 56 of the ’507 Patent and it
`
`is my opinion that all of the elements of these claims are disclosed, or at least
`
`taught or suggested, by U.S. Patent No. 5,626,095 (“the ’095 Patent;” Ex.
`
`1010). My opinion is further solidified when one considers as evidence, the
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`experimental results set forth in the Declaration of Mr. Hiroyuki Miura (Ex.
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`1005; “the Miura Decl.”).
`
`11.
`
`I have reviewed claims 42-44, 47-51, 53, 55, and 56 of the ’507 Patent and it
`
`is my opinion that all of the elements of these claims are taught or suggested
`
`by U.S. Patent No. 6,339,171 (“the ’171 Patent;” Ex. 1011).
`
`12.
`
`It is also my opinion that all of the elements of claims 42-44, 47-51, 53, 55,
`
`and 56 of the ’507 Patent are taught or suggested by U.S. Patent No.
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`6,339,171 (Ex. 1011; “the ’171 Patent”), alone, or in the alternative, in
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`combination with the ’095 Patent and Akinori (Ex. 1012/1013).
`
`13.
`
`It is also my opinion that all of the elements of claims 42-44, 47-51, 53, and
`
`55-57 of the ’507 Patent are taught or suggested by the ’171 Patent in
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`combination with the ’095 Patent and Akinori and Japanese Patent
`
`Application No. 2000-72712 (“JP 2000-72712”). An English Translation of
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`JP 2000-72712 (“JP ’712”) is referenced in the following discussion.
`
`14. The Miura Declaration provides further information, as described below.
`
`Level of Skill in the Art
`
`15.
`
`I am informed that the ’507 Patent has a priority date of March 2, 2004, which
`
`is the filing date of the ’420 Application. I recognize that when considering
`
`the understanding of a skilled scientist – as it relates to the ’507 Patent – I
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`should consider the skilled scientist as of this priority date. For simplicity
`
`herein, I use “in March 2004,” and the like, to mean as of March 2, 2004, the
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`effective filing date of the ’507 Patent.
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`16.
`
`In March 2004, one of ordinary skill in the art would have generally
`
`understood acetic acid production on an industrial scale including the
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`distillation processes and extraction processes that are used in acetic acid or
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`acetic anhydride production. The person of ordinary skill in the art would
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`have understood chemical reactions in general, and, particularly, the primary
`
`reactions and the side-reactions associated with acetic acid production. While
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`the person of ordinary skill in the art may have an advanced degree (M.S. or
`
`Ph.D.) in chemistry or chemical engineering, such is not necessarily required.
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`A chemist or chemical engineer with a BSc honours degree and
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`approximately five years of time in an industrial setting producing acetic acid,
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`acetic anhydride, or related chemicals, would also have the requisite training
`
`and understanding of the nuances of large scale chemical production to be a
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`person of ordinary skill in the art in this context
`
`17. Thus, there is no particular degree requirement. The person of ordinary skill
`
`in the art may be a qualified chemist or chemical engineer, however
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`separations experience, an understanding of industrial-scale processes, and
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`experience in the production of acetic acid, acetic anhydride, or related
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`chemicals, is required.
`
`The Claims of the ’507 Patent
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`18. The Claims of the ’507 Patent recite:
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`42. A process for separating a mixture comprising water,
`acetic acid, methyl iodide, methyl acetate, methanol, and
`at least one permanganate reducing compound (PRC),
`said process comprising the steps of:
`
`(a) distilling the mixture to separate the mixture into a
`plurality of streams, at least one of said streams being a
`PRC enriched overhead stream comprising dimethyl
`ether; and
`
`(b) extracting the PRC enriched overhead stream with
`water to produce an aqueous stream comprising said at
`least one PRC, and a raffinate stream comprising methyl
`iodide,
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`wherein step (b) comprises at least two consecutive
`extraction steps, each extraction step comprising
`contacting the PRC enriched overhead stream with a water
`stream and separating therefrom said aqueous stream
`comprising said at least one PRC and said raffinate stream
`comprising methyl iodide, wherein a fresh water stream is
`used in each discrete extraction stage; or
`
`wherein step (b) comprises at least two consecutive
`extraction steps, each extraction step comprising
`contacting the PRC enriched overhead stream with a water
`stream and separating therefrom said aqueous stream
`comprising said at least one PRC and said raffinate stream
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`comprising methyl iodide, wherein a single water stream
`passes through each of said discrete extraction stages in
`series; or
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`wherein step (b) comprises contacting the PRC enriched
`overhead stream with a water stream and separating
`therefrom said aqueous stream comprising said at least
`one PRC and said raffinate stream comprising methyl
`iodide using a continuous contacting extractor; or a
`combination thereof.
`
`43. The method of claim 42, wherein said PRC enriched
`overhead stream comprises an amount of dimethyl ether in
`excess of any dimethyl ether present in the mixture
`comprising water, acetic acid, methyl iodide, methyl
`acetate, methanol, and at least one PRC.
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`44. The process of claim 42, wherein said at least one PRC
`comprises acetaldehyde.
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`47. The process of claim 42, further comprising the steps
`of:
`
`performing a liquid-vapor phase separation on an effluent
`of a methanol carbonylation reactor to form a vapor phase
`and a liquid phase;
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`distilling the vapor phase to form a first overhead and a
`liquid product stream comprising acetic acid; and
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`condensing at least a portion of the first overhead to
`provide said mixture comprising water, acetic acid,
`methyl iodide, methyl acetate, methanol, and at least one
`PRC, and
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`wherein at least a portion of said raffinate stream is
`recycled directly or indirectly back into said methanol
`carbonylation reactor.
`
`48. The process of claim 47 wherein said at least one PRC
`comprises acetaldehyde
`
`49. The method of claim 48, wherein sufficient
`acetaldehyde
`is removed from said PRC enriched
`overhead stream to maintain a concentration of propionic
`acid of less than about 400 parts per million by weight in
`said liquid product stream.
`
`50. The method of claim 48, wherein sufficient
`acetaldehyde
`is removed from said PRC enriched
`overhead stream to maintain a concentration of propionic
`acid of less than about 250 parts per million by weight in
`said liquid product stream.
`
`51. The method of claim 42, wherein said distillation step
`(a) further comprises the step of adding water to
`distillation step (a) in an amount sufficient to produce
`dimethyl ether from a portion of the mixture during said
`distillation step (a).
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`53. The method of claim 42, wherein said distillation step
`(a) comprises distillation using a single distillation
`column.
`
`55. The method of claim 42, wherein said dimethyl ether
`is present in said PRC enriched overhead stream at a
`concentration sufficient to produce each of said aqueous
`streams comprising said at least one PRC, wherein each
`have a methyl iodide concentration of less than 1.8 wt %.
`
`56. The method of claim 42, wherein said dimethyl ether
`is present in said PRC enriched overhead stream at a
`concentration sufficient to produce said aqueous stream
`comprising said at least one PRC having a methyl iodide
`concentration between about 1.8 wt % and 0.5 wt %.
`
`57. The method of claim 42, wherein said dimethyl ether
`is present in said PRC enriched overhead stream at a
`concentration sufficient to produce each of said aqueous
`streams comprising said at least one PRC, wherein each
`have a methyl iodide concentration of less than or equal to
`about 0.5 wt %.
`
`19. As I will describe below, it is my opinion that the person of ordinary skill in
`
`the art would have found that prior to March 2004, and at least as of the
`
`publication dates of the ’095 and ’171 Patent, the methods of claims 42-44,
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`47-51, 53, and 55-57 were known in the art and to those of ordinary skill in the
`
`art.
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`Acetic Acid Production
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`20. As I understand the technology presented in the ’507 Patent, it is directed to
`
`the production of acetic acid. Specifically, the process is a variation on the
`
`Monsanto process. Both Celanese and Daicel licensed their original process
`
`from Monsanto. The Monsanto process was developed for the production of
`
`acetic acid by the rhodium-catalyzed carbonylation of methanol. (see
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`Akinori, English translation, page 7). The ’507 Patent describes the
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`production of acetic acid at col. 1, lines 13-21 as:
`
`This invention relates to an improved process for the
`removal of permanganate reducing compounds and alkyl
`iodides formed by the carbonylation of methanol in the
`presence of a Group VIII metal carbonylation catalyst.
`More specifically, this invention relates to an improved
`process for reducing and/or removing precursors of
`permanganate reducing compounds and alkyl iodides
`from intermediate streams during the formation of acetic
`acid by said carbonylation processes.
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`21. Specifically, the ’507 Patent provides for a process for the purification of
`
`acetic acid, after its production, by the removal of permanganate reducing
`
`compound and alkyl iodides. Refer to ’507, col. 2, lines 30-36 and 45-49.
`
`Permanganate reducing compounds, or PRC’s include materials such as
`
`acetaldehyde, acetone, methyl ethyl ketone, butyraldehyde, crotonaldehyde,
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`2-ethyl crotonaldehyde, and 2-ethyl butyraldehyde and the like, and the aldol
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`condensation products thereof. Refer to ’507, col. 2, lines 30-36 and 45-49.
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`22. At col. 4 lines 12 to 26, the ’507 Patent describes a process for producing
`
`acetic acid that includes the following steps: (a) reacting methanol,… with
`
`carbon monoxide…. (b) separating the products of the reaction into a volatile
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`product phase that contains acetic acid, methyl iodide, water, and
`
`permanganate reducing compounds (PRC’s), and a less volatile phase
`
`containing the catalyst and acetic acid; (c) distilling the volatile product phase
`
`to yield a purified product and a first overhead that contains organic iodide,
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`water, acetic acid, and unreacted methanol; (d) distilling at least a portion of
`
`the first overhead to produce a second overhead containing methyl iodide,
`
`water, C2-12 alkyl iodides, PRC’s and DME. Claim 42 focuses on a process for
`
`separating a mixture comprising water, acetic acid, methyl iodide, methyl
`
`acetate, methanol, and at least one permanganate reducing compound (PRC).
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`The methanol is unreacted methanol from the Step (a) described above (i.e.,
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`(a) reacting methanol,…). See ’507 Patent col. 4, l. 23.
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`23. Apart from the claims this is the only place where the first overhead is
`
`mentioned. From this context “first overhead” clearly refers to the stream
`
`labelled 28 emanating from the top of column 14 in Figure 1 and 2.
`
`24. At col. 8, lines 1-24, the ’507 Patent provides a more detailed explanation as:
`
`The present invention may broadly be considered as an
`improved process
`for distilling PRC’s, primarily
`aldehydes and alkyl iodides, from a vapor phase acetic
`acid stream, such as the overhead from a light ends
`distillation column or a combined light-ends/drying
`column. The vapor phase stream is distilled and then
`twice extracted to remove PRC’s. An especially preferred
`method of removing aldehydes and alkyl iodides from a
`first vapor phase acetic acid stream, and reducing levels of
`propionic acid in the product, includes the following steps:
`a) condensing the first vapor phase acetic acid stream in a
`first condenser and biphasically separating it to form a
`first heavy liquid phase product and a first light liquid
`phase product; b) distilling the first light liquid phase
`product in a first distillation column to form a second
`vapor phase acetic acid product stream which is enriched
`with aldehydes and alkyl iodides with respect to said first
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`vapor phase acetic acid stream; c) condensing the second
`vapor phase stream in a second condenser to form a
`second liquid phase product; d) distilling the second liquid
`phase product in a second distillation column to form a
`third vapor phase stream; e) condensing the third vapor
`phase stream and extracting the condensed stream with
`water to remove residual acetaldehyde therefrom; and f)
`extracting the extracted condensed stream with water to
`remove additional residual acetaldehyde therefrom.
`
`25. The specification further points out that while the light phase of the first
`
`overhead is preferred, the heavy or light phase may be used, as provided at
`
`col. 8, lines 34-39:
`
`Either phase of the light ends overhead may be
`subsequently distilled to remove the PRC’s and primarily
`the acetaldehyde component of the stream, although it is
`preferred to remove PRC’s from the light phase (30)
`because it has been found that the concentration of
`acetaldehyde is somewhat greater in that phase.
`
`26. Although the concentration of acetaldehyde in the light aqueous phase is
`
`likely to be greater than in the heavy methyl iodide phase the quantity of
`
`acetaldehyde available in the light phase may be insufficient, perhaps only
`
`one sixth of that in the heavy phase. Celanese recognized this issue in the
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`’171 Patent and the ’507 Patent and recycled large amounts of water from
`
`stream 46 to compensate. Refer the ’507 Patent col. 9, lines 24-30.
`
`27. Figure 1 of the ’507 Patent is indicated as depicting the method of the prior
`
`art, while Figure 2 is indicated as depicting the claimed methods. The only
`
`difference between Figures 1 and 2 of the ’507 Patent is the incorporation of
`
`an additional extractor (25) and streams flowing to and from the additional
`
`extractor (25). Further, step (a) of claim 42 of the ’507 Patent should be
`
`considered to be admitted prior art as well, because it is merely describing a
`
`distillation that is done according to Figure 1 of the ’171 Patent.
`
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`28. Acetic acid is produced in a reactor at a temperature of between 150 and 250
`
`ºC. (’507 Patent, col. 7, lines. 4 and 5). A liquid product having dissolved
`
`gases from the reactor is directed to a flasher (not depicted) that removes the
`
`catalyst as a base stream. (’507 Patent, col. 7, lines 46-59). The dissolved
`
`gases, consisting of carbon monoxide, methane, hydrogen, and carbon
`
`dioxide leave the flasher as an overhead stream which is directed to the “light
`
`ends” or “splitter column” 14 (pictured). Id. Exiting light ends column 14 is
`
`stream 28 which is directed to decanter 16. (’507, col. 7, lines 64-65). The
`
`light ends phase (or light phase) 30 is then further distilled. (’507, col. 7, lines
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`65-67, and col. 8, lines 42-50).
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`29. With regard to claim 42 and the description that the “PRC enriched overhead
`
`stream,” the ’507 Patent mentions “stream 28, containing PRC’s,” “light
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`phase (30) is directed to column 18, which serves to form a second vapor
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`phase (36) enriched in aldehydes…” and “stream 52 containing PRC's” as a
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`distillation product from column 22. Thus, a broadest reasonable
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`interpretation of “PRC enriched overhead stream” would include “a stream
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`containing PRC’s.
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`30. Claim 42 recites the term “raffinate stream.” As set forth in the claim, the
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`“raffinate stream” is formed by extracting the PRC enriched overhead stream
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`with water to produce an aqueous stream comprising said at least one PRC,
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`and a raffinate stream comprising methyl iodide. The term “raffinate” is not
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`defined in the specification of the ’507 Patent. Instead, the person of ordinary
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`skill in the art must rely on industry standard definitions, which would
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`indicate that the term is related to the phase that does not contain the extracted
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`component of an extraction.
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`31.
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`In terms of Figure 2 of the ’507 Patent, there are two extractors described by
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`reference numbers 27 (“the first extractor”) and 25 (“the second extractor”).
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`See col. 10, line 56 to col. 11, line 2. The second raffinate is designated in
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`Figure 2 by reference number 72. The second raffinate, 72 (“raffinate
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`stream”), is then split and recycled to the reactor (72) and to a distillation
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`column 22, as stream 68. See Fig. 2. It is noteworthy that stream 68 is not
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`discussed or disclosed in the specification of the ’507 Patent, other than
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`appearing in Figure 2.
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`32. Because the first and second aqueous extract streams are only produced upon
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`extraction, i.e. by an extractor, the first aqueous extract stream is designated
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`by reference number 64 (“aqueous extract stream”) (Ex. 1002, col. 10, l. 58),
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`and the second aqueous extract stream is designated by referenced number 70
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`(“aqueous extract stream”). (Ex. 1002, col. 11, l. 4).
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`33.
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`It should also be noted that a raffinate is the extraction phase that contains less
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`of the extracted component after an extraction. For example, the Oxford
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`Dictionary defines raffinate as “[t]he refined fraction which results after
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`removal of impurities by solvent extraction, spec. in oil refining.” Such a
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`definition comports well with the examples used in the ’507 Patent. For
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`example, at col. 10, ll. 58-62, the ’507 Patent states:
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`The aqueous extract stream 64 leaves the extractor 27
`from the top thereof. This PRC-rich, and in particular,
`acetaldehyde-rich aqueous phase is directed to waste
`treatment. Also exiting the extractor is raffinate stream 66
`containing methyl iodide.
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`34. Accordingly, it is clear that a raffinate is the fraction of the extraction that
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`contains methyl iodide. However, claim 42 recites, in the first two of the three
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`“wherein” clauses, that the extraction comprises at least two consecutive
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`extraction steps, and each extraction step comprises “contacting the PRC
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`enriched overhead stream with a water stream and separating therefrom said
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`aqueous stream comprising said at least one PRC and said raffinate stream
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`comprising methyl iodide.” My interpretation of this language is that the
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`extractors are operated in series with respect to the extract feed. The feed to
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`the first extractor is the PRC enriched overhead stream and the feed to the
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`second extractor is the raffinate stream from the first extractor. The raffinate
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`from these two extractors is the liquid phase consisting primarily of methyl
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`iodide which contains less of the PRC than the original extract feed.
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`35. Claim 42 also recites the term “aqueous stream comprising said at least one
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`PRC.” As set forth in the claim, the “aqueous stream comprising said at least
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`one PRC” is formed along with a raffinate stream. Again, claim 42 recites, in
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`the first two of the three “wherein” clauses, that the extraction comprises at
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`least two consecutive extraction steps, and each extraction step comprises
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`“contacting the PRC enriched overhead stream with a water stream and
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`separating therefrom said aqueous stream comprising said at least one PRC
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`and said raffinate stream comprising methyl iodide.” In terms of Figure 2 of
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`the ’507 Patent, there are two extractors described by reference numbers 27
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`(“the first extractor”) and 25 (“the second extractor”). (Ex. 1002, col. 10, ll.
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`50-51 and 64). Because the first aqueous extract stream is only produced
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`upon extraction, i.e. by an extractor, the first aqueous extract stream is
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`designated by reference number 64 (“aqueous extract stream”) and the second
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`aqueous extract stream is only produced upon extraction, i.e. by an extractor,
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`the second aqueous extract stream is designated in Figure 2 by reference
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`number 70 (“aqueous extract stream”). See col. 10, l. 58; col. 11, l. 4 and (Ex.
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`1003, ¶ 21). The term “aqueous stream comprising said at least one PRC”
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`includes both the first and second aqueous extract streams.
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`36. Claim 47 recites “at least a portion of said raffinate stream is directly or
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`indirectly recycled back into said methanol carbonylation reactor.” As noted
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`above, the raffinate stream is not limited to a first or second raffinate stream.
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`Furthermore, the recycling may be indirect or direct. Therefore, under a
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`broadest reasonable interpretation, this term should be interpreted as the
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`liquid stream coming from the extractor which contains the lower water and
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`higher methyl iodide concentration (i.e., the stream that is not the aqueous
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`extract) and that this stream is recycled back to the methanol carbonylation
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`reactor either directly or via other equipment or process steps (i.e., indirectly).
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`37. Referring back to FIG. 2 of the ’507 Patent, slip stream 68 is shown recycling
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`the methyl iodide-rich raffinate phase from the second stage aqueous
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`extraction 25 to the distillation column 22, but there is no mention of stream
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`68 in the description.
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`38.
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`It is readily apparent from Figures 1 and 2 of the ’507 Patent, that the only
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`difference between “prior art” Figure 1 and “inventive” Figure 2 is the
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`existence of the second extractor 25, as well as connectors thereto, 66, 70, and
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`72. This difference is depicted as one additional extraction step in the bottom
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`right corner of Figure 2.
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`39. Thus, the sole differences between Figure 1 and Figure 2 may be realized by
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`simply focusing on the bottom right corner of the two figures. As shown in
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`Figure 2, slipstream 68 recycles part of the second raffinate 72 back into the
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`second distillation column 22. Indeed the description of Figure 1 and Figure 2
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`merge into each other. There is no mention of the additional extraction step
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`with regard to Figure 2, but in the description of Figure 1 (the prior art) the
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`additional water extraction step is included. For example:
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`…e) condensing the third vapor phase stream and
`extracting the condensed stream with water to remove
`residual acetaldehyde therefrom; and f) extracting the
`extracted condensed stream with water to remove
`additional residual acetaldehyde therefrom.
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`Refer to ’507 Patent Col. 8, lines 20 to 23). The ’507 Patent also describes
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`raffinate stream 66 as being extracted with additional water in a second
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`extractor 25. Refer to ’507 Patent Col. 10 line